Triazole-Containing [FeFe] Hydrogenase Mimics: Synthesis and Electrocatalytic Behavior

Merinero, Alba D.; Collado, Alba; Casarrubios, Luis; Gómez Gallego, Mar; Ramírez de Arellano, Carmen; Caballero, Antonio; Zapata Fernández, Fabiola; Sierra, Miguel A.

Por favor, use este identificador para citar o enlazar este ítem: https://doi.org/10.1021/acs.inorgchem.9b02813

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Campo DC	Valor	Lengua/Idioma
dc.contributor.author	Merinero, Alba D.	-
dc.contributor.author	Collado, Alba	-
dc.contributor.author	Casarrubios, Luis	-
dc.contributor.author	Gómez Gallego, Mar	-
dc.contributor.author	Ramírez de Arellano, Carmen	-
dc.contributor.author	Caballero, Antonio	-
dc.contributor.author	Zapata Fernández, Fabiola	-
dc.contributor.author	Sierra, Miguel A.	-
dc.contributor.other	Facultades, Departamentos, Servicios y Escuelas::Departamentos de la UMU:: Química Orgánica	es
dc.date.accessioned	2024-02-07T08:51:38Z	-
dc.date.available	2024-02-07T08:51:38Z	-
dc.date.issued	2019-12-02	-
dc.identifier.citation	Inorganic Chemistry 58 (23), 2019:16267−16278	es
dc.identifier.issn	Print: 0020-1669	-
dc.identifier.issn	Electronic: 1520-510X	-
dc.identifier.uri	http://hdl.handle.net/10201/138825	-
dc.description	©2019. This manuscript version is made available under the CC-BY 4.0 license http://creativecommons.org/licenses/by-nc-nd/4.0/ This document is the Accepted, version of a Published Work that appeared in final form in Inorganic Chemistry. To access the final edited and published work see https://doi.org/10.1021/acs.inorgchem.9b02813	-
dc.description.abstract	Through a Cu-catalyzed Huisgen cycloaddition between terminal alkynes and azides (CuAAC) reaction, azide [(μ-SCH2)2N(4- N3C6H4)Fe2(CO)6] has demonstrated to be a robust and versatile reagent able to incorporate the [(μ-SR)2Fe2(CO)6] fragment on a wide range of substrates, ranging from aromatic compounds to nucleosides, metallocenes, or redox and luminescent markers. The [FeIFeI]/[Fe0FeI] and [Fe0FeI]/[Fe0Fe0] reduction potentials of the triazole derivatives prepared are comparable to those of other aminodithiolate (adt) Fe−Fe hydrogenase mimics. The presence of the triazole linker influences the electrochemical behavior of these complexes depending on the strength of the acid employed.	es
dc.format	application/pdf	es
dc.format.extent	12	es
dc.language	eng	es
dc.publisher	American Chemical Society	es
dc.relation	CTQ2016-77555-C2-1-R and CTQ2016-81797-REDC (Programa Redes Consolider) from the MINECO (Spain) and from Fundación Ramón Areces (CIVP18A3938)	es
dc.rights	info:eu-repo/semantics/openAccess	es
dc.rights	Attribution-NoCommercial-NoDerivatives 4.0 Internacional	-
dc.rights.uri	http://creativecommons.org/licenses/by-nc-nd/4.0/	-
dc.subject	Triazole	es
dc.subject	Hydrogenase Mimics	-
dc.subject	Electrocatalytic	-
dc.subject.other	CDU::5 - Ciencias puras y naturales::54 - Química::547 - Química orgánica	es
dc.title	Triazole-Containing [FeFe] Hydrogenase Mimics: Synthesis and Electrocatalytic Behavior	es
dc.type	info:eu-repo/semantics/article	es
dc.identifier.doi	https://doi.org/10.1021/acs.inorgchem.9b02813	-
Aparece en las colecciones:	Artículos: Química Orgánica

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